#------------------------------------------------------------------------------ #$Date: 2025-03-26 01:38:22 +0200 (Wed, 26 Mar 2025) $ #$Revision: 298582 $ #$URL: file:///home/coder/svn-repositories/cod/cif/7/25/01/7250176.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/ # # All data on this site have been placed in the public domain by the # contributors. # data_7250176 loop_ _publ_author_name 'Ravi, Sasikala' 'Priyadharsan, R. Rameshbabu' 'Karthikeyan, Subramanian' 'Pannippara, Mehboobali' 'Al-Sehemi, Abdullah G.' 'Moon, Dohyun' 'Anthony, Savarimuthu Philip' _publ_section_title ; Synthesis of dual state emissive twisted donor-acceptor fluorophores: tunable fluorescence and self-reversible mechanofluorochromism ; _journal_name_full CrystEngComm _journal_paper_doi 10.1039/D4CE01317D _journal_year 2025 _chemical_formula_moiety 'C31 H23 N3 O3' _chemical_formula_sum 'C31 H23 N3 O3' _chemical_formula_weight 485.52 _chemical_name_systematic 'ethyl (E)-2-cyano-3-(2-(2-cyanophenoxy)-4-(diphenylamino) phenyl)acrylate' _space_group_crystal_system monoclinic _space_group_IT_number 14 _space_group_name_Hall '-P 2yn' _space_group_name_H-M_alt 'P 1 21/n 1' _atom_sites_solution_hydrogens geom _audit_creation_method SHELXL-2019/3 _audit_update_record ; 2024-12-19 deposited with the CCDC. 2025-03-25 downloaded from the CCDC. ; _cell_angle_alpha 90 _cell_angle_beta 97.19(3) _cell_angle_gamma 90 _cell_formula_units_Z 4 _cell_length_a 7.5180(15) _cell_length_b 36.519(7) _cell_length_c 9.0830(18) _cell_measurement_reflns_used 130337 _cell_measurement_temperature 220(2) _cell_measurement_theta_max 30.000 _cell_measurement_theta_min 0.401 _cell_volume 2474.1(9) _computing_cell_refinement 'HKL3000sm(Otwinowski & Minor, 1997)' _computing_data_collection 'PAL BL2D-SMDC Program(Shin et.al, 2016)' _computing_data_reduction 'HKL3000sm(Otwinowski & Minor, 1997)' _computing_molecular_graphics 'DIAMOND 4(Putx&Brandenburg, 2014)' _computing_publication_material 'publCIF(Westrip, 2010)' _computing_structure_refinement 'SHELXL-2018(Sheldrick, 2018)' _computing_structure_solution 'SHELXT-2018(Sheldrick, 2018)' _diffrn_ambient_temperature 220(2) _diffrn_measured_fraction_theta_full 0.970 _diffrn_measured_fraction_theta_max 0.946 _diffrn_measurement_device_type 'Rayonix MX225HS CCD area detector' _diffrn_measurement_method 'omega scan' _diffrn_radiation_type synchrotron _diffrn_radiation_wavelength 0.700 _diffrn_reflns_av_R_equivalents 0.0712 _diffrn_reflns_av_unetI/netI 0.0603 _diffrn_reflns_Laue_measured_fraction_full 0.970 _diffrn_reflns_Laue_measured_fraction_max 0.946 _diffrn_reflns_limit_h_max 9 _diffrn_reflns_limit_h_min -9 _diffrn_reflns_limit_k_max 48 _diffrn_reflns_limit_k_min -48 _diffrn_reflns_limit_l_max 12 _diffrn_reflns_limit_l_min -12 _diffrn_reflns_number 22303 _diffrn_reflns_point_group_measured_fraction_full 0.970 _diffrn_reflns_point_group_measured_fraction_max 0.946 _diffrn_reflns_theta_full 24.835 _diffrn_reflns_theta_max 28.000 _diffrn_reflns_theta_min 2.197 _diffrn_source 'PLSII 2D bending magnet' _exptl_absorpt_coefficient_mu 0.082 _exptl_absorpt_correction_T_max 1.000 _exptl_absorpt_correction_T_min 0.883 _exptl_absorpt_correction_type empirical _exptl_absorpt_process_details 'HKL3000sm Scalepack(Otwinowski et.al,2003)' _exptl_crystal_colour yellow _exptl_crystal_density_diffrn 1.303 _exptl_crystal_description plate _exptl_crystal_F_000 1016 _exptl_crystal_size_max 0.039 _exptl_crystal_size_mid 0.028 _exptl_crystal_size_min 0.005 _refine_diff_density_max 0.220 _refine_diff_density_min -0.256 _refine_diff_density_rms 0.043 _refine_ls_extinction_coef 0.0252(17) _refine_ls_extinction_expression Fc^*^=kFc[1+0.001xFc^2^\l^3^/sin(2\q)]^-1/4^ _refine_ls_extinction_method 'SHELXL-2019/2 (Sheldrick 2019)' _refine_ls_goodness_of_fit_ref 1.018 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 336 _refine_ls_number_reflns 5903 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.018 _refine_ls_R_factor_all 0.1111 _refine_ls_R_factor_gt 0.0546 _refine_ls_shift/su_max 0.001 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.0596P)^2^+0.3236P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.1190 _refine_ls_wR_factor_ref 0.1413 _reflns_Friedel_coverage 0.000 _reflns_number_gt 3349 _reflns_number_total 5903 _reflns_threshold_expression 'I > 2\s(I)' _cod_data_source_file d4ce01317d2.cif _cod_data_source_block SPA944 _cod_original_sg_symbol_H-M 'P 21/n' _cod_database_code 7250176 _shelx_shelxl_version_number 2019/3 _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _shelx_estimated_absorpt_t_min 0.997 _shelx_estimated_absorpt_t_max 1.000 _shelx_res_file ; TITL SPA944 in P2(1)/n SPA944.res created by SHELXL-2019/3 at 11:28:17 on 19-Mar-2024 CELL 0.70000 7.5180 36.5190 9.0830 90.000 97.191 90.000 ZERR 4.000 0.0015 0.0073 0.0018 0.000 0.030 0.000 LATT 1 SYMM 1/2-X, 1/2+Y, 1/2-Z SFAC C H N O DISP C 0.0030 0.0016 10.98 DISP H 0.0000 0.0000 0.67 DISP N 0.0059 0.0032 18.71 DISP O 0.0105 0.0059 30.82 UNIT 124 92 12 12 OMIT -9 0 5 OMIT 7 13 6 OMIT -8 28 3 OMIT -3 56 TEMP -53 SIZE 0.039 0.028 0.005 L.S. 15 BOND $H LIST 4 ACTA PLAN 15 MERG 2 CONF FMAP 2 WGHT 0.059600 0.323600 EXTI 0.025220 FVAR 0.59638 O1 4 0.610498 0.573354 0.409404 11.00000 0.04599 0.02537 = 0.07113 -0.00804 -0.01887 0.00633 O2 4 0.020488 0.601463 0.268259 11.00000 0.05070 0.03964 = 0.08510 0.00772 -0.01202 -0.00443 O3 4 -0.050668 0.656586 0.172199 11.00000 0.03830 0.04322 = 0.05795 0.00624 -0.00871 0.00194 N1 3 1.026783 0.649072 0.720472 11.00000 0.04222 0.02534 = 0.05101 0.00344 -0.01142 -0.00316 N2 3 0.285454 0.717356 0.252138 11.00000 0.06858 0.04139 = 0.05759 0.00612 -0.01171 -0.00484 N3 3 0.731169 0.533954 0.089616 11.00000 0.06222 0.05618 = 0.08417 -0.00480 -0.00804 0.00253 C1 1 1.120111 0.619122 0.793990 11.00000 0.03949 0.02736 = 0.04372 -0.00020 -0.00705 -0.00180 C2 1 1.303653 0.616298 0.796638 11.00000 0.04183 0.03542 = 0.05478 -0.00034 -0.00475 -0.00389 AFIX 43 H2 2 1.365874 0.633213 0.744136 11.00000 -1.20000 AFIX 0 C3 1 1.395997 0.588384 0.877134 11.00000 0.04272 0.04114 = 0.07404 -0.00607 -0.00875 0.00432 AFIX 43 H3 2 1.521118 0.586684 0.879793 11.00000 -1.20000 AFIX 0 C4 1 1.306759 0.563324 0.952631 11.00000 0.05931 0.03452 = 0.06918 0.00821 -0.01830 0.00760 AFIX 43 H4 2 1.370243 0.544631 1.007625 11.00000 -1.20000 AFIX 0 C5 1 1.124307 0.565683 0.947459 11.00000 0.06136 0.03909 = 0.06392 0.01471 -0.00610 -0.00295 AFIX 43 H5 2 1.062087 0.548216 0.997294 11.00000 -1.20000 AFIX 0 C6 1 1.031495 0.593523 0.869592 11.00000 0.04341 0.03975 = 0.05546 0.00721 -0.00029 -0.00179 AFIX 43 H6 2 0.906463 0.595100 0.867941 11.00000 -1.20000 AFIX 0 C7 1 1.112975 0.684146 0.733887 11.00000 0.03962 0.02555 = 0.04913 0.00160 -0.00501 -0.00066 C8 1 1.171914 0.697939 0.872179 11.00000 0.06794 0.03738 = 0.04680 0.00300 -0.01022 -0.01076 AFIX 43 H8 2 1.147802 0.685346 0.957741 11.00000 -1.20000 AFIX 0 C9 1 1.266680 0.730376 0.884709 11.00000 0.08424 0.03878 = 0.05900 -0.00042 -0.02168 -0.01300 AFIX 43 H9 2 1.308581 0.739689 0.979184 11.00000 -1.20000 AFIX 0 C10 1 1.300094 0.749083 0.760565 11.00000 0.06645 0.03030 = 0.08190 0.00157 -0.00645 -0.01347 AFIX 43 H10 2 1.365578 0.771068 0.769737 11.00000 -1.20000 AFIX 0 C11 1 1.237734 0.735657 0.622678 11.00000 0.07246 0.03340 = 0.06333 0.00493 0.01114 -0.00550 AFIX 43 H11 2 1.259279 0.748596 0.537213 11.00000 -1.20000 AFIX 0 C12 1 1.143594 0.703234 0.609407 11.00000 0.06022 0.03076 = 0.04906 -0.00125 0.00235 -0.00141 AFIX 43 H12 2 1.100212 0.694159 0.514859 11.00000 -1.20000 AFIX 0 C13 1 0.866450 0.644432 0.629243 11.00000 0.03796 0.03053 = 0.04207 0.00036 -0.00502 -0.00187 C14 1 0.819837 0.610568 0.566235 11.00000 0.03842 0.02805 = 0.04965 0.00069 -0.00678 0.00548 AFIX 43 H14 2 0.899746 0.590751 0.581996 11.00000 -1.20000 AFIX 0 C15 1 0.657782 0.606011 0.481261 11.00000 0.03738 0.02798 = 0.04712 -0.00226 -0.00422 -0.00075 C16 1 0.535327 0.634619 0.449981 11.00000 0.03751 0.02821 = 0.04688 -0.00062 -0.00401 0.00130 C17 1 0.589308 0.668958 0.509731 11.00000 0.04374 0.02835 = 0.05158 0.00039 -0.00640 0.00753 AFIX 43 H17 2 0.513495 0.689226 0.487953 11.00000 -1.20000 AFIX 0 C18 1 0.747449 0.673849 0.597948 11.00000 0.04748 0.02587 = 0.04891 -0.00256 -0.00717 0.00233 AFIX 43 H18 2 0.777309 0.697080 0.638254 11.00000 -1.20000 AFIX 0 C19 1 0.681211 0.540800 0.466067 11.00000 0.03319 0.02536 = 0.06952 0.00148 -0.01059 -0.00132 C20 1 0.686330 0.531292 0.612193 11.00000 0.04601 0.04431 = 0.07697 0.00349 0.00007 -0.00433 AFIX 43 H20 2 0.646583 0.547835 0.680332 11.00000 -1.20000 AFIX 0 C21 1 0.750502 0.497107 0.659181 11.00000 0.04777 0.05540 = 0.08644 0.02476 -0.00491 -0.01254 AFIX 43 H21 2 0.755269 0.490559 0.759685 11.00000 -1.20000 AFIX 0 C22 1 0.807230 0.472723 0.559465 11.00000 0.03943 0.03166 = 0.11465 0.02025 -0.01071 -0.00527 AFIX 43 H22 2 0.851750 0.449682 0.592220 11.00000 -1.20000 AFIX 0 C23 1 0.799049 0.481902 0.412829 11.00000 0.03509 0.02866 = 0.09675 0.00031 -0.00945 -0.00024 AFIX 43 H23 2 0.834833 0.464915 0.344552 11.00000 -1.20000 AFIX 0 C24 1 0.737809 0.516368 0.364474 11.00000 0.03011 0.02472 = 0.07745 -0.00173 -0.00892 -0.00267 C25 1 0.733290 0.526437 0.211882 11.00000 0.03891 0.03037 = 0.07825 -0.00746 -0.01015 0.00005 C26 1 0.362836 0.626785 0.370556 11.00000 0.03987 0.02944 = 0.05248 -0.00167 -0.00116 0.00153 AFIX 43 H26 2 0.331691 0.601844 0.368275 11.00000 -1.20000 AFIX 0 C27 1 0.237180 0.648900 0.298433 11.00000 0.04020 0.03260 = 0.04468 -0.00312 -0.00147 0.00168 C28 1 0.264627 0.686815 0.272657 11.00000 0.04179 0.04112 = 0.04033 -0.00191 -0.00739 0.00175 C29 1 0.060463 0.632557 0.244813 11.00000 0.04114 0.03586 = 0.04653 0.00032 -0.00141 0.00293 C30 1 -0.231059 0.642971 0.124307 11.00000 0.03952 0.07377 = 0.07108 0.00702 -0.00757 -0.00394 AFIX 23 H30A 2 -0.224835 0.618568 0.080360 11.00000 -1.20000 H30B 2 -0.298475 0.641107 0.209627 11.00000 -1.20000 AFIX 0 C31 1 -0.320412 0.668234 0.015399 11.00000 0.07556 0.05033 = 0.12902 0.00448 -0.05373 -0.00444 AFIX 137 H31A 2 -0.439966 0.659272 -0.018615 11.00000 -1.50000 H31B 2 -0.252314 0.670113 -0.068212 11.00000 -1.50000 H31C 2 -0.328558 0.692168 0.060376 11.00000 -1.50000 AFIX 0 HKLF 4 REM SPA944 in P2(1)/n REM wR2 = 0.1413, GooF = S = 1.018, Restrained GooF = 1.018 for all data REM R1 = 0.0546 for 3349 Fo > 4sig(Fo) and 0.1111 for all 5903 data REM 336 parameters refined using 0 restraints END WGHT 0.0595 0.3265 REM Highest difference peak 0.220, deepest hole -0.256, 1-sigma level 0.043 Q1 1 0.5589 0.6510 0.4732 11.00000 0.05 0.22 Q2 1 0.4622 0.6270 0.4243 11.00000 0.05 0.21 Q3 1 0.5854 0.6218 0.4634 11.00000 0.05 0.20 Q4 1 -0.3162 0.6641 0.1396 11.00000 0.05 0.18 Q5 1 1.0739 0.6329 0.7578 11.00000 0.05 0.18 Q6 1 1.0559 0.6021 0.7807 11.00000 0.05 0.18 Q7 1 -0.2791 0.6965 -0.0218 11.00000 0.05 0.17 Q8 1 -0.0455 0.6820 0.0811 11.00000 0.05 0.16 Q9 1 0.6388 0.6581 0.5982 11.00000 0.05 0.16 Q10 1 0.7249 0.5571 0.1765 11.00000 0.05 0.16 Q11 1 -0.0122 0.6753 0.2360 11.00000 0.05 0.15 Q12 1 1.3496 0.6028 0.8316 11.00000 0.05 0.15 Q13 1 0.8130 0.6583 0.5995 11.00000 0.05 0.15 Q14 1 0.6741 0.5193 0.4025 11.00000 0.05 0.15 Q15 1 0.2850 0.6005 0.4223 11.00000 0.05 0.15 ; _shelx_res_checksum 66196 loop_ _space_group_symop_operation_xyz 'x, y, z' '-x+1/2, y+1/2, -z+1/2' '-x, -y, -z' 'x-1/2, -y-1/2, z-1/2' loop_ _atom_site_label _atom_site_type_symbol _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_occupancy _atom_site_site_symmetry_order _atom_site_calc_flag _atom_site_refinement_flags_posn _atom_site_refinement_flags_adp _atom_site_refinement_flags_occupancy _atom_site_disorder_assembly _atom_site_disorder_group O1 O 0.6105(2) 0.57335(4) 0.40940(18) 0.0497(4) Uani 1 1 d . . . . . O2 O 0.0205(2) 0.60146(4) 0.2683(2) 0.0602(5) Uani 1 1 d . . . . . O3 O -0.05067(19) 0.65659(4) 0.17220(16) 0.0477(4) Uani 1 1 d . . . . . N1 N 1.0268(2) 0.64907(4) 0.72047(19) 0.0410(4) Uani 1 1 d . . . . . N2 N 0.2855(3) 0.71736(5) 0.2521(2) 0.0575(5) Uani 1 1 d . . . . . N3 N 0.7312(3) 0.53395(6) 0.0896(3) 0.0690(6) Uani 1 1 d . . . . . C1 C 1.1201(3) 0.61912(5) 0.7940(2) 0.0379(5) Uani 1 1 d . . . . . C2 C 1.3037(3) 0.61630(6) 0.7966(2) 0.0449(5) Uani 1 1 d . . . . . H2 H 1.365874 0.633213 0.744136 0.054 Uiso 1 1 calc R U . . . C3 C 1.3960(3) 0.58838(6) 0.8771(3) 0.0540(6) Uani 1 1 d . . . . . H3 H 1.521118 0.586684 0.879793 0.065 Uiso 1 1 calc R U . . . C4 C 1.3068(3) 0.56332(6) 0.9526(3) 0.0566(6) Uani 1 1 d . . . . . H4 H 1.370243 0.544631 1.007625 0.068 Uiso 1 1 calc R U . . . C5 C 1.1243(3) 0.56568(6) 0.9475(3) 0.0560(6) Uani 1 1 d . . . . . H5 H 1.062087 0.548216 0.997294 0.067 Uiso 1 1 calc R U . . . C6 C 1.0315(3) 0.59352(6) 0.8696(2) 0.0468(5) Uani 1 1 d . . . . . H6 H 0.906463 0.595100 0.867941 0.056 Uiso 1 1 calc R U . . . C7 C 1.1130(3) 0.68415(5) 0.7339(2) 0.0390(5) Uani 1 1 d . . . . . C8 C 1.1719(3) 0.69794(6) 0.8722(3) 0.0522(6) Uani 1 1 d . . . . . H8 H 1.147802 0.685346 0.957741 0.063 Uiso 1 1 calc R U . . . C9 C 1.2667(4) 0.73038(6) 0.8847(3) 0.0633(7) Uani 1 1 d . . . . . H9 H 1.308581 0.739689 0.979184 0.076 Uiso 1 1 calc R U . . . C10 C 1.3001(4) 0.74908(6) 0.7606(3) 0.0609(7) Uani 1 1 d . . . . . H10 H 1.365578 0.771068 0.769737 0.073 Uiso 1 1 calc R U . . . C11 C 1.2377(3) 0.73566(6) 0.6227(3) 0.0562(6) Uani 1 1 d . . . . . H11 H 1.259279 0.748596 0.537213 0.067 Uiso 1 1 calc R U . . . C12 C 1.1436(3) 0.70323(6) 0.6094(3) 0.0471(5) Uani 1 1 d . . . . . H12 H 1.100212 0.694159 0.514859 0.056 Uiso 1 1 calc R U . . . C13 C 0.8664(3) 0.64443(5) 0.6292(2) 0.0377(5) Uani 1 1 d . . . . . C14 C 0.8198(3) 0.61057(5) 0.5662(2) 0.0398(5) Uani 1 1 d . . . . . H14 H 0.899746 0.590751 0.581996 0.048 Uiso 1 1 calc R U . . . C15 C 0.6578(3) 0.60601(5) 0.4813(2) 0.0383(5) Uani 1 1 d . . . . . C16 C 0.5353(3) 0.63462(5) 0.4500(2) 0.0383(5) Uani 1 1 d . . . . . C17 C 0.5893(3) 0.66896(5) 0.5097(2) 0.0423(5) Uani 1 1 d . . . . . H17 H 0.513495 0.689226 0.487953 0.051 Uiso 1 1 calc R U . . . C18 C 0.7474(3) 0.67385(5) 0.5979(2) 0.0419(5) Uani 1 1 d . . . . . H18 H 0.777309 0.697080 0.638254 0.050 Uiso 1 1 calc R U . . . C19 C 0.6812(3) 0.54080(5) 0.4661(3) 0.0441(5) Uani 1 1 d . . . . . C20 C 0.6863(3) 0.53129(7) 0.6122(3) 0.0564(6) Uani 1 1 d . . . . . H20 H 0.646583 0.547835 0.680332 0.068 Uiso 1 1 calc R U . . . C21 C 0.7505(3) 0.49711(7) 0.6592(3) 0.0643(7) Uani 1 1 d . . . . . H21 H 0.755269 0.490559 0.759685 0.077 Uiso 1 1 calc R U . . . C22 C 0.8072(3) 0.47272(7) 0.5595(4) 0.0636(8) Uani 1 1 d . . . . . H22 H 0.851750 0.449682 0.592220 0.076 Uiso 1 1 calc R U . . . C23 C 0.7990(3) 0.48190(6) 0.4128(3) 0.0550(6) Uani 1 1 d . . . . . H23 H 0.834833 0.464915 0.344552 0.066 Uiso 1 1 calc R U . . . C24 C 0.7378(3) 0.51637(5) 0.3645(3) 0.0454(5) Uani 1 1 d . . . . . C25 C 0.7333(3) 0.52644(6) 0.2119(3) 0.0507(6) Uani 1 1 d . . . . . C26 C 0.3628(3) 0.62678(6) 0.3706(2) 0.0412(5) Uani 1 1 d . . . . . H26 H 0.331691 0.601844 0.368275 0.049 Uiso 1 1 calc R U . . . C27 C 0.2372(3) 0.64890(5) 0.2984(2) 0.0397(5) Uani 1 1 d . . . . . C28 C 0.2646(3) 0.68682(6) 0.2727(2) 0.0421(5) Uani 1 1 d . . . . . C29 C 0.0605(3) 0.63256(6) 0.2448(2) 0.0418(5) Uani 1 1 d . . . . . C30 C -0.2311(3) 0.64297(8) 0.1243(3) 0.0627(7) Uani 1 1 d . . . . . H30A H -0.224835 0.618568 0.080360 0.075 Uiso 1 1 calc R U . . . H30B H -0.298475 0.641107 0.209627 0.075 Uiso 1 1 calc R U . . . C31 C -0.3204(4) 0.66823(8) 0.0154(4) 0.0906(11) Uani 1 1 d . . . . . H31A H -0.439966 0.659272 -0.018615 0.136 Uiso 1 1 calc R U . . . H31B H -0.252314 0.670113 -0.068212 0.136 Uiso 1 1 calc R U . . . H31C H -0.328558 0.692168 0.060376 0.136 Uiso 1 1 calc R U . . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_23 _atom_site_aniso_U_13 _atom_site_aniso_U_12 O1 0.0460(9) 0.0254(7) 0.0711(11) -0.0080(7) -0.0189(7) 0.0063(6) O2 0.0507(10) 0.0396(9) 0.0851(12) 0.0077(8) -0.0120(8) -0.0044(7) O3 0.0383(8) 0.0432(9) 0.0579(9) 0.0062(7) -0.0087(7) 0.0019(6) N1 0.0422(10) 0.0253(8) 0.0510(10) 0.0034(7) -0.0114(8) -0.0032(7) N2 0.0686(14) 0.0414(12) 0.0576(12) 0.0061(9) -0.0117(10) -0.0048(9) N3 0.0622(15) 0.0562(14) 0.0842(17) -0.0048(12) -0.0080(13) 0.0025(11) C1 0.0395(12) 0.0274(10) 0.0437(11) -0.0002(8) -0.0071(9) -0.0018(8) C2 0.0418(12) 0.0354(11) 0.0548(13) -0.0003(9) -0.0047(10) -0.0039(9) C3 0.0427(13) 0.0411(13) 0.0740(17) -0.0061(11) -0.0087(12) 0.0043(10) C4 0.0593(16) 0.0345(12) 0.0692(16) 0.0082(11) -0.0183(12) 0.0076(10) C5 0.0614(16) 0.0391(13) 0.0639(16) 0.0147(11) -0.0061(12) -0.0029(11) C6 0.0434(13) 0.0398(12) 0.0555(14) 0.0072(10) -0.0003(10) -0.0018(9) C7 0.0396(11) 0.0256(10) 0.0491(12) 0.0016(8) -0.0050(9) -0.0007(8) C8 0.0679(16) 0.0374(12) 0.0468(13) 0.0030(10) -0.0102(12) -0.0108(10) C9 0.0842(19) 0.0388(13) 0.0590(16) -0.0004(11) -0.0217(14) -0.0130(12) C10 0.0665(17) 0.0303(12) 0.0819(18) 0.0016(12) -0.0065(14) -0.0135(11) C11 0.0725(17) 0.0334(12) 0.0633(16) 0.0049(11) 0.0111(13) -0.0055(11) C12 0.0602(14) 0.0308(11) 0.0491(13) -0.0012(9) 0.0023(11) -0.0014(9) C13 0.0380(11) 0.0305(11) 0.0421(11) 0.0004(8) -0.0050(9) -0.0019(8) C14 0.0384(11) 0.0280(10) 0.0497(13) 0.0007(8) -0.0068(9) 0.0055(8) C15 0.0374(11) 0.0280(10) 0.0471(12) -0.0023(8) -0.0042(9) -0.0008(8) C16 0.0375(11) 0.0282(10) 0.0469(12) -0.0006(8) -0.0040(9) 0.0013(8) C17 0.0437(12) 0.0284(10) 0.0516(13) 0.0004(9) -0.0064(10) 0.0075(8) C18 0.0475(13) 0.0259(10) 0.0489(12) -0.0026(8) -0.0072(10) 0.0023(8) C19 0.0332(11) 0.0254(10) 0.0695(15) 0.0015(10) -0.0106(10) -0.0013(8) C20 0.0460(14) 0.0443(13) 0.0770(18) 0.0035(12) 0.0001(12) -0.0043(10) C21 0.0478(15) 0.0554(16) 0.0864(19) 0.0248(14) -0.0049(13) -0.0125(12) C22 0.0394(14) 0.0317(13) 0.115(2) 0.0203(14) -0.0107(14) -0.0053(10) C23 0.0351(12) 0.0287(11) 0.097(2) 0.0003(12) -0.0095(12) -0.0002(9) C24 0.0301(11) 0.0247(10) 0.0775(16) -0.0017(10) -0.0089(10) -0.0027(8) C25 0.0389(13) 0.0304(12) 0.0783(19) -0.0075(11) -0.0102(12) 0.0001(9) C26 0.0399(12) 0.0294(10) 0.0525(13) -0.0017(9) -0.0012(10) 0.0015(8) C27 0.0402(12) 0.0326(11) 0.0447(12) -0.0031(8) -0.0015(9) 0.0017(8) C28 0.0418(12) 0.0411(12) 0.0403(12) -0.0019(9) -0.0074(9) 0.0018(9) C29 0.0411(12) 0.0359(12) 0.0465(12) 0.0003(9) -0.0014(9) 0.0029(9) C30 0.0395(14) 0.0738(18) 0.0711(17) 0.0070(14) -0.0076(12) -0.0039(11) C31 0.076(2) 0.0503(17) 0.129(3) 0.0045(17) -0.0537(19) -0.0044(14) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0030 0.0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0059 0.0032 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0105 0.0059 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle_publ_flag C19 O1 C15 120.25(17) . . ? C29 O3 C30 115.23(18) . . ? C13 N1 C1 121.92(16) . . ? C13 N1 C7 120.69(16) . . ? C1 N1 C7 117.17(16) . . ? C6 C1 C2 118.97(19) . . ? C6 C1 N1 120.99(18) . . ? C2 C1 N1 119.96(18) . . ? C1 C2 C3 119.8(2) . . ? C1 C2 H2 120.1 . . ? C3 C2 H2 120.1 . . ? C4 C3 C2 120.7(2) . . ? C4 C3 H3 119.6 . . ? C2 C3 H3 119.6 . . ? C3 C4 C5 119.5(2) . . ? C3 C4 H4 120.2 . . ? C5 C4 H4 120.2 . . ? C4 C5 C6 120.3(2) . . ? C4 C5 H5 119.8 . . ? C6 C5 H5 119.8 . . ? C5 C6 C1 120.7(2) . . ? C5 C6 H6 119.7 . . ? C1 C6 H6 119.7 . . ? C12 C7 C8 119.9(2) . . ? C12 C7 N1 120.30(19) . . ? C8 C7 N1 119.72(19) . . ? C7 C8 C9 119.6(2) . . ? C7 C8 H8 120.2 . . ? C9 C8 H8 120.2 . . ? C10 C9 C8 120.5(2) . . ? C10 C9 H9 119.8 . . ? C8 C9 H9 119.8 . . ? C9 C10 C11 119.8(2) . . ? C9 C10 H10 120.1 . . ? C11 C10 H10 120.1 . . ? C10 C11 C12 120.0(2) . . ? C10 C11 H11 120.0 . . ? C12 C11 H11 120.0 . . ? C7 C12 C11 120.1(2) . . ? C7 C12 H12 119.9 . . ? C11 C12 H12 119.9 . . ? N1 C13 C14 120.75(18) . . ? N1 C13 C18 120.81(17) . . ? C14 C13 C18 118.44(18) . . ? C15 C14 C13 120.10(18) . . ? C15 C14 H14 119.9 . . ? C13 C14 H14 119.9 . . ? C14 C15 O1 121.91(17) . . ? C14 C15 C16 122.75(18) . . ? O1 C15 C16 115.10(17) . . ? C15 C16 C17 115.93(18) . . ? C15 C16 C26 119.01(18) . . ? C17 C16 C26 124.90(18) . . ? C18 C17 C16 122.24(18) . . ? C18 C17 H17 118.9 . . ? C16 C17 H17 118.9 . . ? C17 C18 C13 120.45(18) . . ? C17 C18 H18 119.8 . . ? C13 C18 H18 119.8 . . ? C20 C19 O1 123.0(2) . . ? C20 C19 C24 120.5(2) . . ? O1 C19 C24 116.3(2) . . ? C19 C20 C21 119.6(2) . . ? C19 C20 H20 120.2 . . ? C21 C20 H20 120.2 . . ? C22 C21 C20 120.3(3) . . ? C22 C21 H21 119.8 . . ? C20 C21 H21 119.8 . . ? C23 C22 C21 120.2(2) . . ? C23 C22 H22 119.9 . . ? C21 C22 H22 119.9 . . ? C22 C23 C24 120.1(2) . . ? C22 C23 H23 119.9 . . ? C24 C23 H23 119.9 . . ? C19 C24 C23 119.2(2) . . ? C19 C24 C25 120.45(19) . . ? C23 C24 C25 120.3(2) . . ? N3 C25 C24 178.9(3) . . ? C27 C26 C16 131.32(19) . . ? C27 C26 H26 114.3 . . ? C16 C26 H26 114.3 . . ? C26 C27 C28 123.72(19) . . ? C26 C27 C29 117.59(19) . . ? C28 C27 C29 118.69(18) . . ? N2 C28 C27 179.5(2) . . ? O2 C29 O3 123.8(2) . . ? O2 C29 C27 123.82(19) . . ? O3 C29 C27 112.29(18) . . ? C31 C30 O3 108.6(2) . . ? C31 C30 H30A 110.0 . . ? O3 C30 H30A 110.0 . . ? C31 C30 H30B 110.0 . . ? O3 C30 H30B 110.0 . . ? H30A C30 H30B 108.3 . . ? C30 C31 H31A 109.5 . . ? C30 C31 H31B 109.5 . . ? H31A C31 H31B 109.5 . . ? C30 C31 H31C 109.5 . . ? H31A C31 H31C 109.5 . . ? H31B C31 H31C 109.5 . . ? loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_distance _geom_bond_site_symmetry_2 _geom_bond_publ_flag O1 C19 1.376(2) . ? O1 C15 1.384(2) . ? O2 C29 1.200(2) . ? O3 C29 1.329(2) . ? O3 C30 1.459(3) . ? N1 C13 1.385(3) . ? N1 C1 1.420(2) . ? N1 C7 1.434(2) . ? N2 C28 1.145(3) . ? N3 C25 1.142(3) . ? C1 C6 1.380(3) . ? C1 C2 1.381(3) . ? C2 C3 1.389(3) . ? C2 H2 0.9400 . ? C3 C4 1.369(3) . ? C3 H3 0.9400 . ? C4 C5 1.369(3) . ? C4 H4 0.9400 . ? C5 C6 1.377(3) . ? C5 H5 0.9400 . ? C6 H6 0.9400 . ? C7 C12 1.372(3) . ? C7 C8 1.374(3) . ? C8 C9 1.380(3) . ? C8 H8 0.9400 . ? C9 C10 1.368(4) . ? C9 H9 0.9400 . ? C10 C11 1.372(3) . ? C10 H10 0.9400 . ? C11 C12 1.377(3) . ? C11 H11 0.9400 . ? C12 H12 0.9400 . ? C13 C14 1.389(3) . ? C13 C18 1.404(3) . ? C14 C15 1.368(3) . ? C14 H14 0.9400 . ? C15 C16 1.398(3) . ? C16 C17 1.406(3) . ? C16 C26 1.432(3) . ? C17 C18 1.360(3) . ? C17 H17 0.9400 . ? C18 H18 0.9400 . ? C19 C20 1.368(3) . ? C19 C24 1.388(3) . ? C20 C21 1.386(3) . ? C20 H20 0.9400 . ? C21 C22 1.375(4) . ? C21 H21 0.9400 . ? C22 C23 1.367(4) . ? C22 H22 0.9400 . ? C23 C24 1.392(3) . ? C23 H23 0.9400 . ? C24 C25 1.430(4) . ? C26 C27 1.349(3) . ? C26 H26 0.9400 . ? C27 C28 1.424(3) . ? C27 C29 1.482(3) . ? C30 C31 1.454(4) . ? C30 H30A 0.9800 . ? C30 H30B 0.9800 . ? C31 H31A 0.9700 . ? C31 H31B 0.9700 . ? C31 H31C 0.9700 . ? loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion_publ_flag C13 N1 C1 C6 -47.1(3) . . . . ? C7 N1 C1 C6 138.3(2) . . . . ? C13 N1 C1 C2 136.1(2) . . . . ? C7 N1 C1 C2 -38.5(3) . . . . ? C6 C1 C2 C3 -1.3(3) . . . . ? N1 C1 C2 C3 175.61(19) . . . . ? C1 C2 C3 C4 0.8(3) . . . . ? C2 C3 C4 C5 0.6(4) . . . . ? C3 C4 C5 C6 -1.4(4) . . . . ? C4 C5 C6 C1 0.9(4) . . . . ? C2 C1 C6 C5 0.4(3) . . . . ? N1 C1 C6 C5 -176.4(2) . . . . ? C13 N1 C7 C12 -51.2(3) . . . . ? C1 N1 C7 C12 123.5(2) . . . . ? C13 N1 C7 C8 131.6(2) . . . . ? C1 N1 C7 C8 -53.7(3) . . . . ? C12 C7 C8 C9 -2.1(4) . . . . ? N1 C7 C8 C9 175.2(2) . . . . ? C7 C8 C9 C10 0.9(4) . . . . ? C8 C9 C10 C11 0.5(4) . . . . ? C9 C10 C11 C12 -0.7(4) . . . . ? C8 C7 C12 C11 1.9(3) . . . . ? N1 C7 C12 C11 -175.3(2) . . . . ? C10 C11 C12 C7 -0.5(4) . . . . ? C1 N1 C13 C14 -21.7(3) . . . . ? C7 N1 C13 C14 152.8(2) . . . . ? C1 N1 C13 C18 158.5(2) . . . . ? C7 N1 C13 C18 -27.0(3) . . . . ? N1 C13 C14 C15 177.32(19) . . . . ? C18 C13 C14 C15 -2.8(3) . . . . ? C13 C14 C15 O1 176.1(2) . . . . ? C13 C14 C15 C16 2.0(3) . . . . ? C19 O1 C15 C14 28.0(3) . . . . ? C19 O1 C15 C16 -157.37(19) . . . . ? C14 C15 C16 C17 0.8(3) . . . . ? O1 C15 C16 C17 -173.74(19) . . . . ? C14 C15 C16 C26 -174.8(2) . . . . ? O1 C15 C16 C26 10.6(3) . . . . ? C15 C16 C17 C18 -2.8(3) . . . . ? C26 C16 C17 C18 172.6(2) . . . . ? C16 C17 C18 C13 1.9(3) . . . . ? N1 C13 C18 C17 -179.19(19) . . . . ? C14 C13 C18 C17 1.0(3) . . . . ? C15 O1 C19 C20 47.7(3) . . . . ? C15 O1 C19 C24 -136.5(2) . . . . ? O1 C19 C20 C21 176.4(2) . . . . ? C24 C19 C20 C21 0.7(3) . . . . ? C19 C20 C21 C22 -0.6(4) . . . . ? C20 C21 C22 C23 -0.7(4) . . . . ? C21 C22 C23 C24 1.8(3) . . . . ? C20 C19 C24 C23 0.4(3) . . . . ? O1 C19 C24 C23 -175.55(18) . . . . ? C20 C19 C24 C25 -179.6(2) . . . . ? O1 C19 C24 C25 4.4(3) . . . . ? C22 C23 C24 C19 -1.6(3) . . . . ? C22 C23 C24 C25 178.4(2) . . . . ? C15 C16 C26 C27 -163.4(2) . . . . ? C17 C16 C26 C27 21.3(4) . . . . ? C16 C26 C27 C28 7.8(4) . . . . ? C16 C26 C27 C29 -171.6(2) . . . . ? C30 O3 C29 O2 1.6(3) . . . . ? C30 O3 C29 C27 -176.31(19) . . . . ? C26 C27 C29 O2 3.8(3) . . . . ? C28 C27 C29 O2 -175.6(2) . . . . ? C26 C27 C29 O3 -178.32(18) . . . . ? C28 C27 C29 O3 2.3(3) . . . . ? C29 O3 C30 C31 -165.2(2) . . . . ?